A main purpose of this paper is to examine the origin and mechanism of nonlinear optical activity in solution. For this purpose, within the dipole-dipole formalism of SFG, we study the nonCondon effect and the effect of the breakdown of the Born-Oppenheimer approximation. We find that in order to determine which mechanism is responsible for this SFG it is necessary to compare the SFG band-shape functions on surfaces and in solutions.


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    Titel :

    Investigation of sum-frequency generation of chiral molecules in solutions


    Beteiligte:
    Hayashi, M. (Autor:in) / Lin, S.H. (Autor:in) / Shen, Y.R. (Autor:in)


    Erscheinungsdatum :

    2003-01-01


    Format / Umfang :

    45317 byte




    Medientyp :

    Aufsatz (Konferenz)


    Format :

    Elektronische Ressource


    Sprache :

    Englisch



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